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He would scowl when he didn't get his way.

to make a facial expression that shows displeasure or anger, typically by lowering the eyebrows and tightening the lips.
She would scowl at the bad news.
Don't scowl; smile for the picture.
He began to scowl in frustration.
scowl in anger
scowl with displeasure
scowl at someone
frown
grimace
glare